VLC file? Like an audio file? There should be an exe file, are you using Winrar to extract it? The exe for me is the very last file named
Yandere Limit Sleepover.exe if it is coming up as an VLC file, you may have somehow changed your default .exe loading program. A way to fix this, is to save the folder to a place on your computer, open the folder and find Yandere Limit Sleepover.exe (VLC in your case) and rename VLC to exe. Also I'm not sure if you are on Mac, if so you may only be able to run the HTML version I have up on the main page here https://windgeargames.itch.io/yandere-limit-sleepover.
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Not sure what the issue is Wind... I'm on pc using windows 10... I'll try and download it once again and see what happens if I send it to a zip file... best thing I can think of. Also my pc runs browser game very laggy now... it's an old model so I'm guessing that's the issue. So I couldn't run the browser version :(