OK after more experimentation I'm realizing it's not that I need a sprite sheet, it's that the assets don't use a consistent grid size, or a traditional 2:1 tile size (32x16, 64x32, etc.). I'm finding cell sizes to be around 161x85, with some variance in the y-dimension. Buildings and props don't adhere to a grid system, so you can't add them to your tile-map easily.
The assets are gorgeous and well-made, just want to give a word of warning for game devs attempting to drop these into a traditional 2:1 iso setup. It is not straightforward and you will get aliasing artifacts due to things not being a power of 2.