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Why does it say "Cannot be uncursed"?

Does that mean it can't ever be unequipped, or can't be collected as infinite?

The former.

So if I gather 4 of them they will become infinite? or will they keep cluttering up the loot drops?

I still need to figure out how the infinite system will work with items like that (there are also items that loop between different forms). Obviously it's not the plan that they keep showing up.